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Received:20 March 2025,
Revised:2025-10-31,
Accepted:05 November 2025,
Online First:02 February 2026,
Published:2026-12
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Michele Cotrufo, Luca Carletti, Adam Overvig, et al. Nonlinear nonlocal metasurfaces[J]. eLight, 2026, 6.
Michele Cotrufo, Luca Carletti, Adam Overvig, et al. Nonlinear nonlocal metasurfaces[J]. eLight, 2026, 6. DOI: 10.1186/s43593-025-00116-7.
Nonlinear metasurfaces have been enabling unprecedented control over light generation and wave mixing
demonstrating enhanced wavefront control
beam shaping and steering of nonlinear light waves. However
the design and operation of nonlinear metasurfaces have been for the most part limited to localized modes
fundamentally limiting the overall nonlinearity enhancement of such devices. Periodic structures supporting extended lattice resonances can realize much larger quality-factor resonances
and hence stronger nonlinearity enhancement
but they are fundamentally limited in their wavefront shaping capabilities
due to their high symmetry. Nonlocal metasurfaces have been recently introduced in linear settings to support highly delocalized resonant modes that can promote very large quality factors
yet without requiring periodicity
hence providing also local control over the wavefront. Here
we extend the powerful features of nonlocal metasurfaces to nonlinear phenomena
experimentally demonstrating nonlinear nonlocal metasurfaces that simultaneously support high quality factor modes
and hence strong nonlinearity enhancement
as well as a spatially varying geometric phase tailored over a subwavelength scale. We show how nonlinear nonlocal metasurfaces can at the same time enhance light-matter interactions
boosting nonlinear conversion efficiency
and enable precise subwavelength control over the wavefront of the generated light. Using this platform
we demonstrate a silicon metasurface for beam steering of third-harmonic generation in the visible. Our results show control over the polarization and steering angle of the third-harmonic signal
extending the framework of diffractive nonlocal metasurfaces to nonlinear optics
and pave the way for the development of nanoscale nonlinear devices with unparalleled control over the optical properties of generated light.
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