Applications of ultrafast nano-spectroscopy and nano-imaging with tip-based microscopy

Zhichen Zhao; Vasily Kravtsov; Zerui Wang; Zhou Zhou; Linyuan Dou; Di Huang; Zhanshan Wang; Xinbin Cheng; Markus B. Raschke; Tao Jiang

doi:10.1186/s43593-024-00079-1

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Applications of ultrafast nano-spectroscopy and nano-imaging with tip-based microscopy

eLight 2025年5卷

Review | Updated：2025-04-15

- Applications of ultrafast nano-spectroscopy and nano-imaging with tip-based microscopy
- Applications of ultrafast nano-spectroscopy and nano-imaging with tip-based microscopy
- Affiliations：
- Author bio：
  
  h chengxb@tongji.edu.cn
  j markus.raschke@colorado.edu
  k tjiang@tongji.edu.cn
- Funds：
  
  National Natural Science Foundation of China;Science and Technology Commission of Shanghai Municipality;Priority 2030 Federal Academic Leadership Program;National Science Foundation;U.S. Department of Energy, Office of Basic Sciences, Division of Material Sciences and Engineering
- DOI：10.1186/s43593-024-00079-1
  中图分类号：
- 收稿日期：2024-09-01，
  
  修回日期：2024-10-20，
  
  录用日期：2024-11-05，
  
  网络出版日期：2025-01-13，
  
  纸质出版日期：2025-12
- Accepted：
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Applications of ultrafast nano-spectroscopy and nano-imaging with tip-based microscopy[J]. eLight, 2025,5.

Zhichen Zhao, Vasily Kravtsov, Zerui Wang, et al. Applications of ultrafast nano-spectroscopy and nano-imaging with tip-based microscopy[J]. Elight, 2025, 5.
Applications of ultrafast nano-spectroscopy and nano-imaging with tip-based microscopy[J]. eLight, 2025,5. DOI： 10.1186/s43593-024-00079-1.

Zhichen Zhao, Vasily Kravtsov, Zerui Wang, et al. Applications of ultrafast nano-spectroscopy and nano-imaging with tip-based microscopy[J]. Elight, 2025, 5. DOI： 10.1186/s43593-024-00079-1.

摘要

Abstract

Innovation in microscopy has often been critical in advancing both fundamental science and technological progress. Notably

the evolution of ultrafast near-field optical nano-spectroscopy and nano-imaging has unlocked the ability to image at spatial scales from nanometers to ångströms and temporal scales from nanoseconds to femtoseconds. This approach revealed a plethora of fascinating light-matter states and quantum phenomena

including various species of polaritons

quantum phases

and complex many-body effects. This review focuses on the working principles and state-of-the-art development of ultrafast tip-enhanced and near-field microscopy

integrating diverse optical pump-probe methods across the terahertz (THz) to ultraviolet (UV) spectral ranges. It highlights their utility in examining a broad range of materials

including two-dimensional (2D)

organic molecular

and hybrid materials. The review concludes with a spatio-spectral-temporal comparison of ultrafast nano-imaging techniques

both within already well-defined domains

and offering an outlook on future developments of ultrafast tip-based microscopy and their potential to address a wider range of materials.

关键词

Keywords

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